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Apart from Girls' Generation's activities, Taeyeon also appeared in several solo appearances.
She first contributed her vocals to "7989" (featuring Kangta), a track taken from both Girls' Generation's eponymous debut album (2007) and Kangta's fourth studio album, Eternity (2008).
Thereafter, Taeyeon started gaining popularity through her various television soundtracks, having recorded "If" for the KBS2's drama Hong Gil Dong (2008) and "Can You Hear Me" for MBC's drama Beethoven Virus (2009).
Taeyeon briefly dabbled with an acting career by making a theatrical debut.
Ahn recalled his impression of the latter song: "I was surprised at how well Taeyeon could sing.
This is a rather mature song, so I would be lying if I said I didn’t have my doubts, but she blew me away.
I was moved to tears listening to her singing." Following Taeyeon's working relationship with him from the drama Beethoven Virus (2008), musical director Lee Pil-ho was determined to collaborate with her again on his MBC's melodrama The King 2 Hearts (2012) soundtrack, by having her record the main theme song "Missing You Like Crazy".
It peaked at number two on South Korea's Gaon Album Chart and its title track sold over one million digital copies.
Her second extended play, Why (2016), charted at number one and yielded two Gaon Digital Chart top-ten singles "Starlight" and "Why".